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Other research infrastructure

Single particle reactor

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BEST - Bioenergy and Sustainable Technologies GmbH

Graz | Website

Open for Collaboration

Short Description

Characterization of the thermal decomposition behavior of single biomass particles (pellets, chips).

Operating Conditions / Application Range
• Temperature range: 200 – 1,050 °C
• Variable atmospheres (from 100% N₂ to air)

Continuous data acquisition of:
• Surface and core temperatures of the particle/sample
• Mass loss of the particle over the entire thermochemical conversion process
• Composition of product gases using FT-IR, ND-IR, FID, CLD, and thermal conductivity analyzers
• Concentrations of released aerosol-forming elements using ICP-MS

Discontinuous sampling for tar analysis

Contact Person

Walter Haslinger

Research Services

• Fundamental studies of thermochemical conversion (pyrolysis, gasification, combustion) of biogenic particles
• Continuous measurement of O₂, CO, CO₂, H₂O, H₂, OGC, NO, NO₂, HCN, NH₃, HCl, SO₂, and various hydrocarbons during thermal conversion
• Online detection of the release of inorganic aerosol-forming elements (e.g. S, Cl, K, Na, Zn, and Pb) by coupling the reactor to an inductively coupled plasma mass spectrometer (ICP-MS)

Methods & Expertise for Research Infrastructure

The reactor system was designed to investigate thermal conversion processes (gasification, combustion, pyrolysis) of individual biogenic particles. It enables targeted experiments under defined gas atmospheres (typically mixtures of N₂ and air or pure N₂) at temperatures up to 1050 °C. A wide range of analytical instruments can be coupled to the reactor.
Through connection with an inductively coupled plasma mass spectrometer (ICP-MS), real-time data on the release of inorganic aerosol-forming elements (e.g. S, Cl, K, Na, Zn, and Pb) can be generated.

To date, the reactor has been successfully applied to study the time-resolved release of relevant aerosol-forming elements from various biomass pellets at three different temperatures. These data contribute to a better understanding of ash-forming element release and serve as a basis for model development. The system has also proven effective in describing pyrolysis processes of individual particles.

Allocation to research infrastructure

Analytical Laboratory for Solid Biofuels and Process Products

Terms of Use

The single particle reactor is a self-development, where trained staff is needed to carry out the test runs. Research objectives as well as other tests can be adapted individually if necessary. Specific conditions of use on request.

Reference Projects

BRISK - Biofuels Research Infrastructure for Sharing Knowledge, Duration: 2011-2015, FP7 INFRA-2011-1.1.15, www.briskeu.com

BRISK II, Biofuels Research Infrastructure for Sharing Knowledge II, Duration: 2017- 2023, Horizon 2020, www.brisk2.eu

Reference Publications

Sommersacher P., Kienzl N., Brunner T., Obernberger I. Simultaneous online determination of S, Cl, K, Na, Zn and Pb release from a single particle during biomass combustion Part 1: Experimental setup-implementation and evaluation. Energy and Fuels 2015, 29, 6734-6746

Sommersacher P., Kienzl N., Brunner T., Obernberger I. Simultaneous online determination of S, Cl, K, Na, Zn and Pb release from a single particle during biomass combustion Part 2: Results from test runs with spruce and straw pellets. Energy Fuels, 2016, 30 (4), pp 3428–3440

Anca-Couce A., Sommersacher P., Scharler R., Hochenauer C. Detailed Reaction Schemes and Product Characterization Applied to Pyrolysis of a Single Spruce Particle. In proceedings of the 24th European Biomass Conference and Exhibition, June 2016, Amsterdam

Sommersacher P., Kienzl N., Hochenauer C. Online determination of the release of S, Cl, K, Na, Zn and Pb during combustion of a single Miscanthus pellet. In proceedings of the 26th Confernence: impacts of fuel quality on power production, September 2016, Prague

Contact

Walter Haslinger
+43 5 02378-9200
walter.haslinger@best-research.eu
https://www.best-research.eu

Location

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